TY - JOUR
T1 - Wood-Graphene Oxide Composite for Highly Efficient Solar Steam Generation and Desalination
AU - Liu, Keng Ku
AU - Jiang, Qisheng
AU - Tadepalli, Sirimuvva
AU - Raliya, Ramesh
AU - Biswas, Pratim
AU - Naik, Rajesh R.
AU - Singamaneni, Srikanth
N1 - Funding Information:
The authors acknowledge the financial support from the Air Force Office of Scientific Research (S.S., Award # FA9550-15-1-0228; R.R.N., Award # 12RX11COR), AFRL/RH and National Science Foundation (CBET-1604542). The authors thank Prof. Lihong Wang from Department of Biomedical Engineering at Washington University in St. Louis for providing access to IR camera and the Nano Research Facility (NRF) at Washington University in St. Louis for providing access to electron microscopy facilities.
Publisher Copyright:
© 2017 American Chemical Society.
PY - 2017/3/1
Y1 - 2017/3/1
N2 - Solar steam generation is a highly promising technology for harvesting solar energy, desalination and water purification. We introduce a novel bilayered structure composed of wood and graphene oxide (GO) for highly efficient solar steam generation. The GO layer deposited on the microporous wood provides broad optical absorption and high photothermal conversion resulting in rapid increase in the temperature at the liquid surface. On the other hand, wood serves as a thermal insulator to confine the photothermal heat to the evaporative surface and to facilitate the efficient transport of water from the bulk to the photothermally active space. Owing to the tailored bilayer structure and the optimal thermo-optical properties of the individual components, the wood-GO composite structure exhibited a solar thermal efficiency of ∼83% under simulated solar excitation at a power density of 12 kW/m2. The novel composite structure demonstrated here is highly scalable and cost-efficient, making it an attractive material for various applications involving large light absorption, photothermal conversion and heat localization.
AB - Solar steam generation is a highly promising technology for harvesting solar energy, desalination and water purification. We introduce a novel bilayered structure composed of wood and graphene oxide (GO) for highly efficient solar steam generation. The GO layer deposited on the microporous wood provides broad optical absorption and high photothermal conversion resulting in rapid increase in the temperature at the liquid surface. On the other hand, wood serves as a thermal insulator to confine the photothermal heat to the evaporative surface and to facilitate the efficient transport of water from the bulk to the photothermally active space. Owing to the tailored bilayer structure and the optimal thermo-optical properties of the individual components, the wood-GO composite structure exhibited a solar thermal efficiency of ∼83% under simulated solar excitation at a power density of 12 kW/m2. The novel composite structure demonstrated here is highly scalable and cost-efficient, making it an attractive material for various applications involving large light absorption, photothermal conversion and heat localization.
KW - desalination
KW - graphene oxide
KW - photothermal
KW - solar steam
KW - wood
UR - https://www.scopus.com/pages/publications/85014271767
U2 - 10.1021/acsami.7b01307
DO - 10.1021/acsami.7b01307
M3 - Article
C2 - 28151641
AN - SCOPUS:85014271767
SN - 1944-8244
VL - 9
SP - 7675
EP - 7681
JO - ACS Applied Materials and Interfaces
JF - ACS Applied Materials and Interfaces
IS - 8
ER -