TY - JOUR
T1 - Societal shifts due to COVID-19 reveal large-scale complexities and feedbacks between atmospheric chemistry and climate change
AU - Laughner, Joshua L.
AU - Neu, Jessica L.
AU - Schimel, David
AU - Wennberg, Paul O.
AU - Barsanti, Kelley
AU - Bowman, Kevin W.
AU - Chatterjee, Abhishek
AU - Croes, Bart E.
AU - Fitzmaurice, Helen L.
AU - Henze, Daven K.
AU - Kim, Jinsol
AU - Kort, Eric A.
AU - Liu, Zhu
AU - Miyazaki, Kazuyuki
AU - Turner, Alexander J.
AU - Anenberg, Susan
AU - Avise, Jeremy
AU - Cao, Hansen
AU - Crisp, David
AU - De Gouw, Joost
AU - Eldering, Annmarie
AU - Fyfe, John C.
AU - Goldberg, Daniel L.
AU - Gurney, Kevin R.
AU - Hasheminassab, Sina
AU - Hopkins, Francesca
AU - Ivey, Cesunica E.
AU - Jones, Dylan B.A.
AU - Liu, Junjie
AU - Lovenduski, Nicole S.
AU - Martin, Randall V.
AU - McKinley, Galen A.
AU - Ott, Lesley
AU - Poulter, Benjamin
AU - Ru, Muye
AU - Sander, Stanley P.
AU - Swart, Neil
AU - Yung, Yuk L.
AU - Zeng, Zhao Cheng
N1 - Publisher Copyright:
© 2021 National Academy of Sciences. All rights reserved.
PY - 2021/11/16
Y1 - 2021/11/16
N2 - The COVID-19 global pandemic and associated government lockdowns dramatically altered human activity, providing a window into how changes in individual behavior, enacted en masse, impact atmospheric composition. The resulting reductions in anthropogenic activity represent an unprecedented event that yields a glimpse into a future where emissions to the atmosphere are reduced. Furthermore, the abrupt reduction in emissions during the lockdown periods led to clearly observable changes in atmospheric composition, which provide direct insight into feedbacks between the Earth system and human activity. While air pollutants and greenhouse gases share many common anthropogenic sources, there is a sharp difference in the response of their atmospheric concentrations to COVID-19 emissions changes, due in large part to their different lifetimes. Here, we discuss several key takeaways from modeling and observational studies. First, despite dramatic declines in mobility and associated vehicular emissions, the atmospheric growth rates of greenhouse gases were not slowed, in part due to decreased ocean uptake of CO2 and a likely increase in CH4 lifetime from reduced NOx emissions. Second, the response of O3 to decreased NOx emissions showed significant spatial and temporal variability, due to differing chemical regimes around the world. Finally, the overall response of atmospheric composition to emissions changes is heavily modulated by factors including carbon-cycle feedbacks to CH4 and CO2, background pollutant levels, the timing and location of emissions changes, and climate feedbacks on air quality, such as wildfires and the ozone climate penalty.
AB - The COVID-19 global pandemic and associated government lockdowns dramatically altered human activity, providing a window into how changes in individual behavior, enacted en masse, impact atmospheric composition. The resulting reductions in anthropogenic activity represent an unprecedented event that yields a glimpse into a future where emissions to the atmosphere are reduced. Furthermore, the abrupt reduction in emissions during the lockdown periods led to clearly observable changes in atmospheric composition, which provide direct insight into feedbacks between the Earth system and human activity. While air pollutants and greenhouse gases share many common anthropogenic sources, there is a sharp difference in the response of their atmospheric concentrations to COVID-19 emissions changes, due in large part to their different lifetimes. Here, we discuss several key takeaways from modeling and observational studies. First, despite dramatic declines in mobility and associated vehicular emissions, the atmospheric growth rates of greenhouse gases were not slowed, in part due to decreased ocean uptake of CO2 and a likely increase in CH4 lifetime from reduced NOx emissions. Second, the response of O3 to decreased NOx emissions showed significant spatial and temporal variability, due to differing chemical regimes around the world. Finally, the overall response of atmospheric composition to emissions changes is heavily modulated by factors including carbon-cycle feedbacks to CH4 and CO2, background pollutant levels, the timing and location of emissions changes, and climate feedbacks on air quality, such as wildfires and the ozone climate penalty.
KW - Air quality
KW - COVID-19
KW - Earth system
KW - Greenhouse gases
KW - Mitigation
UR - http://www.scopus.com/inward/record.url?scp=85119265882&partnerID=8YFLogxK
U2 - 10.1073/pnas.2109481118
DO - 10.1073/pnas.2109481118
M3 - Article
C2 - 34753820
AN - SCOPUS:85119265882
SN - 0027-8424
VL - 118
JO - Proceedings of the National Academy of Sciences of the United States of America
JF - Proceedings of the National Academy of Sciences of the United States of America
IS - 46
M1 - e2109481118
ER -