Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion

  • Ioannis Giannakis
  • , Justin Leshen
  • , Mariam Kavai
  • , Sheng Ran
  • , Chang Jong Kang
  • , Shanta R. Saha
  • , Y. Zhao
  • , Z. Xu
  • , J. W. Lynn
  • , Lin Miao
  • , L. Andrew Wray
  • , Gabriel Kotliar
  • , Nicholas P. Butch
  • , Pegor Aynajian

Research output: Contribution to journalArticlepeer-review

Abstract

Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whether Kondo lattice can develop inside the magnetically ordered phase. Using spectroscopic imaging with scanning tunneling microscope, complemented by neutron scattering, x-ray absorption spectroscopy, and dynamical mean field theory, we probe the electronic states in antiferromagnetic USb2. We visualize a large gap in the antiferromagnetic phase within which Kondo hybridization develops below ~80 K. Our calculations indicate the antiferromagnetism and Kondo lattice to reside predominantly on different f-orbitals, promoting orbital selectivity as a new conception into how these phenomena coexist in heavy-fermions. Finally, at 45 K, we find a novel first order-like transition through abrupt emergence of nontrivial 5f-electronic states that may resemble the “hidden-order” phase of URu2Si2.

Original languageEnglish
Article numbereaaw9061
JournalScience Advances
Volume5
Issue number10
DOIs
StatePublished - Oct 18 2019

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