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Hydrogen-bond-mediated aglycone delivery (HAD) and related methods in carbohydrate chemistry

Research output: Chapter in Book/Report/Conference proceedingChapterpeer-review

Abstract

The stereocontrol of glycosylation reactions is a constant struggle in the field of synthetic carbohydrate chemistry. The application of the picoloyl (Pico) substituent can offer numerous stereocontrolling avenues. The most popular application is the Hydrogen-bond-mediated Aglycone Delivery (HAD) method that provides excellent selectivity in the glycosylation of a variety of sugar substrates. The HAD method relies on the formation of an intermolecular hydrogen bond between the nitrogen atom of the Pico substituent on the glycosyl donor with the hydroxy group of the glycosyl acceptor. This interaction provides a facial preference for the nucleophilic attack and hence provides powerful stereocontrol for the glycosidic bond formation. Surveyed herein is the application of the Pico group to stereoselective synthesis of carbohydrates.

Original languageEnglish
Title of host publicationChemical and Biological Approaches
EditorsAmelia Pilar Rauter, Thisbe K. Lindhorst, Yves Queneau
PublisherRoyal Society of Chemistry
Pages93-116
Number of pages24
ISBN (Electronic)9781788013680
DOIs
StatePublished - 2021

Publication series

NameCarbohydrate Chemistry
Volume44
ISSN (Print)2041-353X
ISSN (Electronic)1465-1963

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