TY - JOUR
T1 - Characterizing elemental, equivalent black, and refractory black carbon aerosol particles
T2 - A review of techniques, their limitations and uncertainties
AU - Lack, Daniel A.
AU - Moosmüller, Hans
AU - McMeeking, Gavin R.
AU - Chakrabarty, Rajan K.
AU - Baumgardner, Darrel
PY - 2014/1
Y1 - 2014/1
N2 - Elemental-, equivalent black-and refractory blackcarbon are terms that have been defined in order to dissect the more general term, black carbon, into its component parts related to its specific chemical and optical properties and its impact on climate and health. Recent publications have attempted to clarify the meaning of these terms with respect to their environmental impact, particularly on climate. Here, we focus on the measurement aspects, reviewing the most commonly implemented techniques for the direct and indirect derivation of black carbon properties, their strengths, limitations, and uncertainties, and provide a non-exhaustive bibliography where the reader can find more detailed information. This review paper is designed as a guide for those wishing to learn about the current state of black carbon measurement instrumentation, how calibration is carried out, when one instrument may have the advantage over another, and where new techniques are needed to fill important knowledge gaps.
AB - Elemental-, equivalent black-and refractory blackcarbon are terms that have been defined in order to dissect the more general term, black carbon, into its component parts related to its specific chemical and optical properties and its impact on climate and health. Recent publications have attempted to clarify the meaning of these terms with respect to their environmental impact, particularly on climate. Here, we focus on the measurement aspects, reviewing the most commonly implemented techniques for the direct and indirect derivation of black carbon properties, their strengths, limitations, and uncertainties, and provide a non-exhaustive bibliography where the reader can find more detailed information. This review paper is designed as a guide for those wishing to learn about the current state of black carbon measurement instrumentation, how calibration is carried out, when one instrument may have the advantage over another, and where new techniques are needed to fill important knowledge gaps.
KW - Aerosols
KW - Chemical sensors
KW - Optical sensors
KW - Particulates
KW - Thermalmethods
UR - http://www.scopus.com/inward/record.url?scp=84892999330&partnerID=8YFLogxK
U2 - 10.1007/s00216-013-7402-3
DO - 10.1007/s00216-013-7402-3
M3 - Review article
AN - SCOPUS:84892999330
SN - 1618-2642
VL - 406
SP - 99
EP - 122
JO - Analytical and Bioanalytical Chemistry
JF - Analytical and Bioanalytical Chemistry
IS - 1
ER -