An all solid-state narrow bandwidth optical parametric oscillator and its applications to the high resolution spectroscopy of free radicals

  • O. V. Chekhlov
  • , J. A.J. Fitzpatrick
  • , K. N. Rosser
  • , C. M. Western
  • , S. H. Ashworth

Research output: Contribution to journalConference articlepeer-review

6 Scopus citations

Abstract

The paper describes the design, performance and illustrative spectroscopic applications of a high power, pulsed, injection seeded, narrow bandwidth and continuously tuneable optical parametric oscillator (OPO) based on two β-barium borate (BBO) nonlinear crystals. A ring cavity OPO was injection seeded with an external cavity diode laser in the spectral range 755-855 nm. The OPO generated high power transform limited nanosecond light pulses in this range and, simultaneously, at 606-667 nm. Spectral parameters of the OPO were investigated as a function of pump power for two different cavity lengths. A bandwidth of ∼120 MHz (0.004 cm-1) in the visible has been achieved with a 40-cm-long cavity. The potential of the OPO system is demonstrated by recording high resolution sub-Doppler spectra in the UV of PF and C3 radicals in a pulsed supersonic jet expansion.

Original languageEnglish
Pages (from-to)865-876
Number of pages12
JournalJournal of Modern Optics
Volume49
Issue number5-6
DOIs
StatePublished - Apr 15 2002
Event15th UK National Quantum Electronics and Photonics Conference - Glasgow, United Kingdom
Duration: Sep 3 2001Sep 6 2001

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